TY - JOUR
T1 - Liquid phase IR detector based on the photothermal effect of reduced graphene oxide-doped liquid crystals
AU - Adeshina, Mohammad A.
AU - Lee, Hakseon
AU - Mareddi, Bharath Kumar
AU - Kang, Daekyung
AU - Ogunleye, Abdulazeez M.
AU - Kim, Hyunmin
AU - Kim, Taewan
AU - Choi, Muhan
AU - Park, Hongsik
AU - Park, Jonghoo
N1 - Publisher Copyright:
© 2023 The Royal Society of Chemistry.
PY - 2023/1/3
Y1 - 2023/1/3
N2 - Owing to the additional functionalities endowed by nanoparticle dopants, liquid crystals doped with nanoparticles are promising optical materials in a wide range of applications. In this study, we exploited the photothermal effect of reduced graphene oxide (rGO)-doped 5CB nematic liquid crystals (LC-rGO) to develop an infrared (IR) detector that is not only sensitive to IR but also measures the temperature and energy deposited in the detector. We demonstrate that rGO doping in LCs significantly enhances the IR absorption and transforms the light energy into thermal energy through the photothermal effect. The changes in the orientational order and birefringence of the LC-rGO induced by the photothermal effect under IR irradiation were manifested as an instantaneous color change in the white light probe beam. The change in the probe beam intensity was further translated into a temperature change and energy deposited in the detector. We also demonstrated that the external voltage applied to the detector significantly amplifies the photothermal responsivity by compensating for the anchoring energy of the LC. This study proposes a novel technology for detecting IR, temperature, and energy deposited in the detector by means of visible light, which has significant potential for developing large-area and high-resolution IR detectors by exploiting mature liquid crystal display technologies.
AB - Owing to the additional functionalities endowed by nanoparticle dopants, liquid crystals doped with nanoparticles are promising optical materials in a wide range of applications. In this study, we exploited the photothermal effect of reduced graphene oxide (rGO)-doped 5CB nematic liquid crystals (LC-rGO) to develop an infrared (IR) detector that is not only sensitive to IR but also measures the temperature and energy deposited in the detector. We demonstrate that rGO doping in LCs significantly enhances the IR absorption and transforms the light energy into thermal energy through the photothermal effect. The changes in the orientational order and birefringence of the LC-rGO induced by the photothermal effect under IR irradiation were manifested as an instantaneous color change in the white light probe beam. The change in the probe beam intensity was further translated into a temperature change and energy deposited in the detector. We also demonstrated that the external voltage applied to the detector significantly amplifies the photothermal responsivity by compensating for the anchoring energy of the LC. This study proposes a novel technology for detecting IR, temperature, and energy deposited in the detector by means of visible light, which has significant potential for developing large-area and high-resolution IR detectors by exploiting mature liquid crystal display technologies.
UR - http://www.scopus.com/inward/record.url?scp=85147317968&partnerID=8YFLogxK
U2 - 10.1039/d2nr06220h
DO - 10.1039/d2nr06220h
M3 - Article
C2 - 36651184
AN - SCOPUS:85147317968
SN - 2040-3364
VL - 15
SP - 2061
EP - 2066
JO - Nanoscale
JF - Nanoscale
IS - 5
ER -