Removal of NOx at low temperature over mesoporous α-Mn2O3 catalyst

Mi Jin Jeon, Sung Hoon Park, Ji Man Kim, Jong Ki Jeon, Sang Chai Kim, Do Heui Kim, Young Kwon Park

Research output: Contribution to journalArticlepeer-review

13 Scopus citations

Abstract

Low-temperature selective catalytic reduction was carried out over various kinds of manganese oxide (MnOx) catalysts. Mesoporous α-Mn 2O3, commercial bulk Mn2O3, and Mn/SBA-15 were used as the catalyst. The NOx removal performances of the catalysts were compared. Three different amounts of Mn (5, 10, and 15 wt%) were impregnated on SBA-15 to synthesize Mn/SBA-15. The physical and chemical properties of the catalysts were examined by Brunauer-Emmett-Teller, X-ray diffraction, X-ray photoelectron spectroscopy, and H2-temperature programmed reduction analyses. Of all catalysts examined, mesoporous α-Mn2O3 exhibited the highest low-temperature SCR de-NOx efficiency, reaching about 90% at 175 °C. This is attributed to strong reducing ability and high oxygen mobility of mesoporous α-Mn 2O3 and well dispersed Mn2O3 in its mesoporous framework.

Original languageEnglish
Pages (from-to)2527-2531
Number of pages5
JournalJournal of Nanoscience and Nanotechnology
Volume14
Issue number3
DOIs
StatePublished - Mar 2014

Keywords

  • DeNOx
  • Mesoporous α-MnO
  • NH-SCR

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