Room-temperature ammonia gas sensing via Au nanoparticle-decorated TiO₂ nanosheets

A high-performance gas sensor operating at room temperature is always favourable since it simplifies the device fabrication and lowers the operating power by eliminating a heater. Herein, we fabricated the ammonia (NH₃) gas sensor by using Au nanoparticle-decorated TiO₂ nanosheets, which were synthesized via two distinct processes: (1) preparation of monolayer TiO₂ nanosheets through flux growth and a subsequent chemical exfoliation and (2) decoration of Au nanoparticles on the TiO₂ nanosheets via hydrothermal method. Based on the morphological, compositional, crystallographic, and surface characteristics of this low-dimensional nano-heterostructured material, its temperature- and concentration-dependent NH₃ gas-sensing properties were investigated. A high response of ~ 2.8 was obtained at room temperature under 20 ppm NH₃ gas concentration by decorating Au nanoparticles onto the surface of TiO₂ nanosheets, which generated oxygen defects and induced spillover effect as well.